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Assessing The Fate of Emerging Contaminants in The Environment
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**Assessing the fate of emerging contaminants in the environment**:
- Réf **ABG-128669**
- Sujet de Thèse
- 17/02/2025
- Contrat doctoral
- Université de Lille
- Lieu de travail- VILLENEUVE D'ASCQ - Les Hauts de France - France
- Intitulé du sujet- Assessing the fate of emerging contaminants in the environment
- Champs scientifiques- Chimie
- Ecologie, environnement
- Mots clés- atmospheric chemistry, contaminants, environment, molecular simulations
**Description du sujet**:
Context
- The presence of emerging contaminants results either from direct emission or from diffuse emissions or re-emissions from contaminated soils or waterbodies. This phenomenon concerns a great diversity of molecules, which originate in human uses or activities releasing semi volatile organic compounds such as tire wear additives or perfluorinated compounds (PFAS). On one side, tire wear particles are a new focus as a form of environmental microplastics, with their role in air pollution expected to grow as tailpipe emissions decrease. On the other side, significant research currently focuses on PFAS due to the growing awareness of their toxicity and emerging regulations that often set their allowable concentrations at extremely low levels (a few parts per trillion, ppt). Despite this, many knowledge gaps remain regarding the environmental fate and transport of these compounds, often referred to as "forever chemicals" because of their environmental persistence. Given the limited reactivity of PFAS, a critical consideration is their partitioning behavior within environmental media. One particularly important aspect is the interaction between PFAS and microplastics, as these compounds are frequently found together due to their anthropogenic origins.
- The main goal of this PhD thesis is to investigate using computational kinetics the atmospheric degradation processes of emerging contaminants at the molecular level unraveling their most favorable pathways, their atmospheric fate and impact to the environment as well as their ecotoxicity towards aquatic species. The goal is to inform the experiments on recommended products to look for, and vice-versa, to support the kinetics and products already identified. This project will also perform within the framework of a larger research program (CPER Ecrin; Labex CaPPA, and CDP AREA). This work will be conducted in close collaboration with the experimental works performed in the group led by Pierre Herckes at Arizona State University (ASU).
**Prise de fonction**:
- 01/10/2025
**Nature du financement**:
- Contrat doctoral
**Précisions sur le financement**:
- Financement thèse labellisée ULille/Région Hauts-de-France/Labex CaPPA
**Présentation établissement et labo d'accueil**:
- Université de Lille
The PC2A is a multidisciplinary research unit, interested in the study of atmospheric and combustion environments. It has a large experience in gas phase and multiphase reactivity and deploys an expertise in environmental chemistry using both experimental and theoretical approaches.
**Site web**:
**Intitulé du doctorat**:
- Doctorat de Chimie
**Pays d'obtention du doctorat**:
- France
**Etablissement délivrant le doctorat**:
- Université de Lille
**Ecole doctorale**:
- 104 : Sciences de la matière, du rayonnement et de l'environnement
Master’s degree or engineering degree in environmental chemistry or physical chemistry with average marks at the first session above 12/20 and only MsC. obtained in 2024 or that will be obtained in 2025. Skills in the field of atmospheric chemistry, molecular simulations (quantum chemistry, molecular dynamics) and chemical kinetics will be appreciated. A good level of English (written/spoken) will be essential (at least B2). A mobility between the University of Lille and American partner is asked. The work will take place at PC2A laboratory of the University of Lille.- 25/04/2025
